
While locked in Arkham, Harley was offered a pardon if she assisted Batman in capturing the Joker and stopping his plans of using a nuclear weapon.
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Afterwards, Harley was part of the mock trial that she and other inmates organized to eliminate Batman in Arkham, but she was defeated along with the rest of the criminals. However, neither of them could stop them and instead, they were captured by Officer Renée Montoya. Their success drew the attention of both Batman and The Joker, who sought them in order to stop their crimes for their own personal reasons. In order to prove herself, Harley went as a solo act, but she met Poison Ivy, with whom she started a strong alliance and a successful crime spree. Īfter a failed robbery, Joker blamed Harley for the event and she was kicked out of the gang. Sidney was arrested and Harley posed as his lawyer, taking him out of prison, but into the grasp of the Joker. Later, Harley played a vital part on Joker's plan to get revenge against Sidney Debris, as he had supposedly killed Batman. Her plan, however, backfired when Batman simultaneously captures her and locates the the power switch to the machine. When Batman showed up, Harley tried to escape by turning on the conveyer belt and bolting, hoping to force Batman to choose between apprehending her or saving the bound and gagged Catwoman. Harley gleefully taunted her captive, who bucked desperately against her bonds, indignantly cussing into her gag. Harley bound and gagged a furious Catwoman, lying her down on a conveyor belt of a cat food processing assembly line. The Clown of Crime instructed Harley to eliminate Catwoman the next night inside a cat food factory. Catwoman appeared in time to save Batman, but she ended up captured by the Joker. On their next caper, they managed to capture Batman and placed him on a deadly trap. The Joker eventually returned and Harley resumed her role as his sidekick. Harley and the rest of Joker's gang were stopped by Batman and subsequently arrested by the Police, but Joker was presumed dead, which made Harley mourn for her lost love. She would later capture Harvey Bullock when the detective found Joker's hideout.

Carl Francis with a binary chemical that would kill him when exposed to the second part of the chemical. These included the plan to copyright the "Joker Fish" and the subsequent murder attempts of a couple of Gotham public officials. After that, she became an accessory in practically all of the Joker's felonious schemes. Batman defeated her after a short-lived bout. Her part of the plan was to deliver a massive cake to the ceremony dressed as a police officer. Harley's first deed was to help the Joker in an attempt on James Gordon's life, by planting a bomb at his testimonial banquet. She broke The Joker out and became his criminal sidekick. This changed Quinzel's way of thinking and The Joker was able to manipulate it using his charismatic and flamboyant behavior. During her sessions with Joker, he behaved as a misunderstood person who just wanted affection. Initially drawn to the "charm" of the patients, she was surprisingly interested by the Joker.

Harleen Quinzel was a former psychiatrist whose life took a fundamental turn when she chose to intern at Arkham Asylum.
